Methanolysis Optimization of Cottonseed Oil to Biodiesel Using Heterogeneous Catalysts

سال انتشار: 1399
نوع سند: مقاله ژورنالی
زبان: انگلیسی
مشاهده: 9

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شناسه ملی سند علمی:

JR_IJCCE-39-4_030

تاریخ نمایه سازی: 17 خرداد 1404

چکیده مقاله:

This paper presented the process optimization for heterogeneous catalysts transesterification of refined cottonseed oil catalyzed by calcium oxide (CaO) and magnesium oxide (MgO) impregnated on Saw Dust Ash (SDA) using Response Surface Methodology Central Composite Design (RSMCCD). The five transesterification process variables studied were: catalyst concentration (۴-۸ wt% oil), methanol/oil molar ratio (۴:۱-۸:۱), reaction temperature (۴۵-۸۵oC), reaction time (۳-۵h), and agitation speed (۲۰۰-۳۰۰rpm). It was revealed that the reaction temperature gave the most significant effect on the yield of Fatty Acid Methyl Ester (FAME), followed by methanol/oil molar ratio. There were also significant interaction effects between catalyst concentration and methanol/oil molar ratio, catalyst concentration and agitation speed, methanol/oil molar ratio and reaction temperature, methanol/oil molar ratio and reaction time, methanol/oil molar ratio and agitation speed, reaction time and agitation speed for CaO/SDA transesterified reaction while for MgO/SDA transesterified reaction the significant interaction effect between variable is methanol/oil molar ratio and reaction time. Based on the optimized conditions, the highest yield of ۹۰% for CaO/SDA transesterified reaction and ۷۷% for MgO/SDA transesterified reaction were predicted using the following variables catalyst concentration, CaO/SDA = ۶wt% and MgO/SDA = ۸wt%, methanol/oil molar ratio = ۶:۱(CaO/SDA) and ۸:۱ (MgO/SDA), reaction temperature = ۶۵oC, reaction time = ۴h and agitation speed = ۲۵۰rpm. Experimental validation of the predicted optimum conditions gave an actual yield of ۸۶% (CaO/SDA) and ۷۳.۳% (MgO/SDA). The small errors between the predicted and actual optimum yield (۴.۷% (CaO/SDA) and ۵.۲% (MgO/SDA)) indicated that the model were valid and accurate in representing the actual experimental values and also in predicting yield at any conditions within the range studied.  The results proved the efficacy of saw dust ash impregnated with CaO and MgO in transesterification reaction.

نویسندگان

Callistus Ude

Department of Chemical Engineering, Michael Okpara University of Agriculture, Umudike, Umuahia, NIGERIA

Okechukwu Dominic Onukwuli

Department of Chemical Engineering, Nnamdi Azikiwe University (NAU), Awka, NIGERIA

Boniface Ugwu

Department of Chemical Engineering, Michael Okpara University of Agriculture, Umudike, Umuahia, NIGERIA

Chinenye Faith Okey-Onyesolu

Department of Chemical Engineering, Nnamdi Azikiwe University (NAU), Awka, NIGERIA

Timothy Ezidinma

Department of Chemical Engineering, Institute of Management & Technology (I.M.T), Enugu, NIGERIA

Paul Ejikeme

Department of Pure and Industrial Chemistry, University of Nigeria, Nsukka, NIGERIA

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