Tetra zole derivatives a s effective inhibitors for the corrosion of steel in ۰.۵ M H ۲SO۴ solution

سال انتشار: 1391
نوع سند: مقاله کنفرانسی
زبان: انگلیسی
مشاهده: 179

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شناسه ملی سند علمی:

ISPTC15_0634

تاریخ نمایه سازی: 11 دی 1400

چکیده مقاله:

Corrosive solutions in the aci dic tetrazol e are more and more e ncountered in industry [۱]. The importa nce of inhibitive protection in acidic solutions is increased by the fact that steels which are more s usceptible to be attacked in aggr essive media, are the commonly exposed metals in industrial environ ments. It is shown that the protective pro pertiesof tetrazole derivatives depen d upon thei r ability to reduce co rrosion rate and are enhanced at higher electro n densities around the nitrogen atoms. Nu merous wo rks have been devoted to the corrosi on inhibiting effect of aqueous soluble tetrazole on meta llic materia ls [۲].The effect of organic nitrogen compounds on the cor rosion behaviour of metallic materials in aggressive solutio ns has bee n well documented [ ۳–۷]. Their choice is based on their low-c ost and stabilit y as corrosion inhibitors for metallic materia ls in acidic media. The most synthesised compo unds are th e nitrogen heterocyclic compoun ds, which are very kno wn to be e xcellent complex or chelate formingsubstances witht metals of transition series. Their adso rption is generally explained by the formation of an adher ent film on the metal surface [۷-۸]. The percentage inhibition efficiency was f ound to increase wit h increasing concentration of inhibito r to reach ۹ ۶% at ۱۰-۳ M. This compound is efficient inhibitor.In th e present w ork, we investig ate the corrosion of steel in ۰.۵M H۲SO۴ by som e newly synthesised tetrazole compo unds. The effect of ad dition of tetrazole derivatives on the corrosion of steel in ۰.۵M H۲SO۴ solution is studied using weight loss measurements, electrochemical pol arisation methods. This study permits to follow the evolution of the inhibitive effect of t etrazole derivatives on steel in ۰.۵M H ۲SO۴. Polarisation measurements show that the tetrazole act as mixed inhibitors. The cathodic curvesind icate that the reduction of proton at the steel surface happens within a pure act ivating mechanism. We note a good agreement between gravimetric, electrochemical polarisationand method s.

نویسندگان

L adan Edjlali

Department of Applied Chemistry, Faculty of Science, Isla mic Azad Uni versity, Tabri z Branch, P.O.Box ۱۶ ۵۵, Tabriz, Ira n

Roghaye h Sadeghz adeh

Department of Applied Chemistry, Faculty of Science, Isla mic Azad Uni versity, Tabri z Branch, P.O.Box ۱۶ ۵۵, Tabriz, Ira n

Hosse in Babazad eh

Department of Applied Chemistry, Faculty of Science, Isla mic Azad Uni versity, Tabri z Branch, P.O.Box ۱۶ ۵۵, Tabriz, Ira n

Parasto farsh foroush

Department of Applied Chemistry, Faculty of Science, Isla mic Azad Uni versity, Tabri z Branch, P.O.Box ۱۶ ۵۵, Tabriz, Ira n